LEON MCNEILL With iEatBrainz the default results can be quite off-the-mark, which requires a lot of care given that iEatBrainz replaces your song's title, artist, album, and track # all in one action. Fine if you really don't know for sure what a song really is, or don't know who sings it -- I myself use iEatBrainz for questionable tracks like that.
I know of no other solution other than MPFreaker which will automatically find and add artwork en masse to your library. Indeed, if you're happy with manually working with each song, all you really need is Safari and iTunes.
(Version 1.2)